Document Type
Article
Publication Date
5-20-2020
Publication Title
Journal of Optical Society of America B
Volume
37
Issue
6
First page number:
1769
Last page number:
1774
Abstract
The second hyperpolarizability (��) of carbon disulfide (CS2) is measured by gas-phase electric-field-induced second-harmonic generation for laser wavelengths in the range 765–1064 nm. The observed hyperpolarizability is decomposed into electronic (����) and vibrational (����) contributions, and the dispersion curve for ���� is extrapolated to the static limit, with the result of ����0=12558±93 atomic units =7.83±0.06×10−61C4m4J−3=6.33±0.0×10−36 esu (Taylor series convention). The results of this experiment agree with other recent nonlinear optical measurements and theoretical calculations.
Disciplines
Atomic, Molecular and Optical Physics
File Format
File Size
424 KB
Language
English
Rights
IN COPYRIGHT. For more information about this rights statement, please visit http://rightsstatements.org/vocab/InC/1.0/
Creative Commons License
This work is licensed under a Creative Commons Attribution 4.0 International License.
Repository Citation
Fernandez, R. N.,
Shelton, D. P.
(2020).
Hyperpolarizability Dispersion Measured for CS2 Vapor.
Journal of Optical Society of America B, 37(6),
1769-1774.
http://dx.doi.org/10.1364/JOSAB.394315